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<p class="MsoTitle"><span style="font-family:"Times New
Roman","serif"">Colloqui
Classe di Scienze<o:p></o:p></span></p>
<p class="MsoTitle" style="text-align:left" align="left"><span
style="font-size:
10.0pt;font-family:"Times New
Roman","serif""><o:p><span
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<h2><span style="font-family:"Times New
Roman","serif";mso-no-proof:yes">Mercoledì
18 dicembre 2013</span><span style="font-family:"Times New
Roman","serif""><o:p></o:p></span></h2>
<p class="MsoNormal" style="margin-left:9.0pt;text-align:center;
line-height:18.0pt;tab-stops:324.0pt" align="center"><span
style="font-size:16.0pt;font-family:
"Times New Roman","serif"">ore <span
style="mso-no-proof:yes">15:00</span><o:p></o:p></span></p>
<p class="MsoNormal" style="margin-left:9.0pt;text-align:center;
line-height:18.0pt;tab-stops:324.0pt" align="center"><span
style="font-size:16.0pt;font-family:
"Times New Roman","serif""><o:p> </o:p></span></p>
<p class="MsoNormal" style="margin-left:9.0pt;text-align:center;
line-height:18.0pt;tab-stops:324.0pt" align="center"><u><span
style="font-size:16.0pt;
font-family:"Times New Roman","serif"">Scuola
Normale Superiore<o:p></o:p></span></u></p>
<p class="MsoNormal" style="margin-left:9.0pt;text-align:center;
line-height:18.0pt;tab-stops:324.0pt" align="center"><span
style="font-size:16.0pt;font-family:
"Times New Roman","serif"">Pisa<o:p></o:p></span></p>
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line-height:18.0pt;tab-stops:324.0pt" align="center"><span
style="font-size:16.0pt;
font-family:"Times New
Roman","serif";mso-ansi-language:EN-US"
lang="EN-US">(Sala Stemmi)<o:p></o:p></span></p>
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style="font-size:10.0pt;font-family:"Times New
Roman","serif";mso-ansi-language:
EN-US" lang="EN-US"><o:p><span style="text-decoration:none"> </span></o:p></span></u></b></p>
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text-autospace:none" align="center"><strong><span
style="font-size:26.0pt">Prof. </span></strong><b><span
style="font-size:26.0pt;font-family:"Times New
Roman","serif"">Massimo Olivucci</span></b><b
style="mso-bidi-font-weight:normal"><span
style="font-size:24.0pt;font-family:
"Times New Roman","serif""><br>
</span></b><i style="mso-bidi-font-style:normal"><span
style="font-family:"Times New
Roman","serif"">Chemistry
Department,Bowling Green State University,Bowling Green, OH
43403 (USA)<br>
Dipartimento di Biotechnologie, Chimica e Farmacia, Università
degli Studi di
Siena, 53100 Siena (Italy)</span></i><b><span
style="font-size:26.0pt;
font-family:"Times New Roman","serif""><o:p></o:p></span></b></p>
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Terrà un seminario
dal titolo:<o:p></o:p></span></p>
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Photobiology to the Design of Vibrationally Coherent
Molecular Devices and Motors”<o:p></o:p></span></b></p>
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text-autospace:none"><span style="font-family:"Times New
Roman","serif";
mso-ansi-language:EN-US" lang="EN-US"><b>Abstract: </b><br>
In the past multi-configurational quantum chemical
computations
coupled with molecular mechanics force fields have been
employed to investigate
spectroscopic, thermal and photochemical properties of visual
pigments. <br>
Here we
show how the same computational technology can nowadays be
used to design,
characterize and ultimately, prepare light-driven molecular
switches which
mimics the photophysics of the visual pigment rhodopsin (Rh)
displayed in
Figure A. When embedded in the protein cavity the chromophore
of Rh undergoes
an ultrafast and coherent photoisomerization. In order to
design a synthetic
chromophore displaying similar properties in common solvents,
we recently
focused on indanylidene-pyrroline (NAIP) systems.</span><span
style="font-size:18.0pt;font-family:"RotisSansSerif","sans-serif";mso-bidi-font-family:
RotisSansSerif;mso-ansi-language:EN-US" lang="EN-US"> </span><span
style="font-family:"Times New
Roman","serif";mso-ansi-language:EN-US"
lang="EN-US">We found
that these systems display light-induced ground state coherent
vibrational
(Figure B) motion similar to the one detected in Rh.
Semiclassical trajectories
provide a mechanistic description of the structural changes
associated to the
observed coherent motion which is shown to be ultimately due
to periodic
changes in the </span><span style="font-family:"Times
New Roman","serif"">π</span><span
style="font-family:"Times New
Roman","serif";mso-ansi-language:EN-US"
lang="EN-US">-conjugation.<o:p></o:p></span></p>
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mso-bidi-font-size:12.0pt;
font-family:TradeGothicPl-CondEighteen;
mso-ascii-font-family:TradeGothicPl-CondEighteen;
mso-hansi-font-family:TradeGothicPl-CondEighteen;}
span.PidipaginaCarattere
{mso-style-name:"Piè di pagina Carattere";
mso-style-unhide:no;
mso-style-locked:yes;
mso-style-link:"Piè di pagina";
mso-ansi-font-size:12.0pt;
mso-bidi-font-size:12.0pt;
font-family:TradeGothicPl-CondEighteen;
mso-ascii-font-family:TradeGothicPl-CondEighteen;
mso-hansi-font-family:TradeGothicPl-CondEighteen;}
span.TitoloCarattere
{mso-style-name:"Titolo Carattere";
mso-style-unhide:no;
mso-style-locked:yes;
mso-style-link:Titolo;
mso-ansi-font-size:24.0pt;
mso-bidi-font-size:24.0pt;
font-family:"New York","serif";
mso-ascii-font-family:"New York";
mso-hansi-font-family:"New York";
font-weight:bold;
text-decoration:underline;
text-underline:single;}
.MsoChpDefault
{mso-style-type:export-only;
mso-default-props:yes;
font-size:10.0pt;
mso-ansi-font-size:10.0pt;
mso-bidi-font-size:10.0pt;}
@page WordSection1
{size:595.0pt 842.0pt;
margin:127.6pt 42.25pt 4.0cm 42.55pt;
mso-header-margin:42.55pt;
mso-footer-margin:48.75pt;
mso-paper-source:0;}
div.WordSection1
{page:WordSection1;}
-->
</style><!--[if gte mso 10]>
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table.MsoNormalTable
{mso-style-name:"Tabella normale";
mso-tstyle-rowband-size:0;
mso-tstyle-colband-size:0;
mso-style-noshow:yes;
mso-style-priority:99;
mso-style-parent:"";
mso-padding-alt:0cm 5.4pt 0cm 5.4pt;
mso-para-margin:0cm;
mso-para-margin-bottom:.0001pt;
mso-pagination:widow-orphan;
font-size:10.0pt;
font-family:"Times New Roman","serif";}
</style>
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